The original lineup of sisters, Barbara and Phyllis Allbut, and Linda Jansen (born Linda Jankowski) had their first hit with "Til" released by Gerry Granahan's Caprice label in 1961. The song was followed up with a less-successful single, "Cry Baby Cry." Jansen left the group in 1962 and was replaced by Peggy Santiglia, formerly of The Delicates.
The group left Smash in 1964 and signed with Congress Records. The group became The Halos, Following a dispute over the ownership of the name "The Angels." Santiglia left the group shortly thereafter and was replaced by Toni Mason. The group released several more singles, none of which charted.
Mason left the group in 1967 and was replaced by Debra Swisher (previously of The Pixies Three), who had recently recorded and released her own version of "Thank You And Goodnight" on the ABC-Paramount Records subsidiary, Boom Records. This lineup resumed using the name "The Angels" and released a handful of singles on RCA Records, with Bernadette Carroll singing lead, and made an appearance on "The Dean Martin Show" before disbanding in 1968. Santiglia and Phyllis and Barbara Allbut regrouped in the early 1970s and released a new single on Polydor Records.
Phyllis Allbut and Santiglia still perform as The Angels, joined occasionally by Barbara Allbut.